Hourly total traffic volumes from counters on I-93 nearest to the study area (Fig. A1) were acquired from MassDOT. Fleet composition during the lockdown was not publicly available for I-93; therefore, we used data from I-90 in Boston (Transportation Data Management System, n.d.). Lockdown-period traffic volumes on other roadways in the study area were not available. Meteorological data collected at Logan International Airport (KBOS) were obtained from the National Centers for Environmental Information (NOAA NCEI, n.d.) and aggregated to hourly resolution. Hourly historical concentrations of BC, NO2 and PM2.5 from regulatory sites in Boston (MassDEP, 2019) were obtained via EPA's AirData and AirNow websites (https://aqs.epa.gov/api; https://docs.airnowapi.org/) and MA Department of Environmental Protection (April 1, 2020 onwards, Leslie Collyer, personal communication, June 5, 2020). Data were obtained for two sites: (a) a site on the shoulder of I-93, just south of Boston, which is part of EPA's near-road network (Von Hillern; ID: 25–025-0044); and (b) a site 6.5 km south of Somerville in Roxbury, which is considered indicative of the urban background (ID: 25–025-0042). See Figs. A2–A3 for locations of these regulatory sites and annual average traffic volumes estimated by the Boston Metropolitan Planning Organization (MassGIS, 2018a) on streets around these sites. Roadway classes were assigned by linking GPS location with MA Executive Office of Transportation - Office of Transportation Planning (EOT-OTP) road data layers (MassGIS, 2018b). Data were analyzed using ArcMap 10.5, R 3.5.1 and 3.6 and MATLAB 2019b.
On-road mobile measurements reflect the local background and on-road emissions by local traffic. Further, to quantify the reduction in traffic contributions to air pollution during the lockdown, we needed to compare lockdown-period data to datasets preceding the pandemic while controlling for day-to-day and seasonal variation in the local background. Therefore, we estimated the local background as the 5th percentile on-road value (similar to several previous mobile monitoring studies (Hudda et al., 2013b; Simon et al., 2020; Hudda et al., 2014)) per road class per lap of the monitoring route. The local traffic contribution component of the total on-road measurement was then quantified by subtracting the estimated background from the mean and median on-road concentration (per road class per lap). Differences between road class and monitoring periods were tested using the non-parametric Wilcoxon rank sum test (significance threshold p = 0.05) because pollutant concentrations were not normally distributed.
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