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Magnetization measurements were performed by a superconducting quantum interference device magnetometer from Quantum Design, MPMS (magnetic property measurement system). Electrical resistivity, Seebeck coefficient, and thermal conductivity were measured using a physical property measurement system (PPMS; Quantum Design) from 10 to 400 K under magnetic fields from 0 to 7 T for all the samples and up to 9 T for selected samples. Magnetic field, electric current, and temperature gradient were all in parallel, as indicated in the inset of Fig. 1C. Hall effect measurements of the Fe2V0.9Cr0.1Al0.9Si0.1 sample were carried out using a square-shaped sample (5 by 5 by 1 mm3) by the PPMS with a current of 10 mA under scanning magnetic field from −7 to 7 T.

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