High-pressure carbon monoxide synthetic method (HiPCO) single-walled CNTs were purchased from Unidym (0.8 to 1.2 nm in diameter and median length of 300 nm; batch no. SP0295). 2,4,6-Trichloro-1,3,5-triazine (cyanuric chloride or triazine), 2,3,3-trimethylindolenine, and 5-nitrosalicylaldehyde were purchased from Sigma-Aldrich. Sodium azide and N-methyl-2-pyrrolidone were purchased from Merck. Solvents and materials were used as they received and without further purifications. The synthesis of the SP-CNTs proceeded in two steps following (25): attachment of the triazine moieties onto the tubes (Trz-CNTs) and subsequent growth of the SP-MC switching moiety on the tubes (SP-CNTs).

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