The bilayer-based 2D perovskite was fabricated by postdipping treatment of the 3D perovskite with a solution of the 2D reagent, FEAI in IPA with a concentration of 30 mM for 10 s. The residue FEAI solution was removed by spin coating, followed by annealing treatment at 120°C for 10 min. The procedure was finished in a nitrogen-filled glovebox.

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