The paramagnetic-to-collinear phase transition at Tcollinear was also measured by differential scanning calorimetry (DSC) for REBaCuFeO5 and YBa1−xSrxCuFeO5 powder samples by using a NETZSCH DSC 204F1 device. Fine powders (mass, ~30 mg) were sealed into aluminum crucibles and heated up to 670 K with a rate of 15 K/min under Ar gas flow. The data were acquired during the heating process (see fig. S2).

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